Reaction Analyses Based on Quaternary Metal/Metal Oxide Catalyst Testing in Micro-Structured Reactors Using Combinatorial High-Throughput Methods for Power-to-Gas Applications

To optimize the Sabatier process, quaternary supported catalyst materials are synthesized and tested. The syntheses are performed by the industrially established, reproducible and automated methods of impregnation and sol–gel synthesis. The screening of the 588 quaternary catalysts is carried out in a specially designed 10-fold parallel gas flow micro-structured reactor as wall catalysts in sequential operation mode at a temperature of T = 573 K and a pressure of p = 15 bar. For the description of the activity, the reaction parameters CO2 conversion, CH4 yield, and CH4/CO2 selectivity are used... Mehr ...